Alkaline COFs with precisely arranged active sites achieved >99% conversion and excellent selectivity in flow Knoevenagel condensation, where transition-state stabilization dominates over sieving effects. This establishes a molecular engineering approach for high-efficiency catalysts via organized active sites in crystalline COF matrices.
W. Tang, R. Zhong, H. Zhao and Z. Lu, Chem. Commun., 2025, Accepted Manuscript , DOI: 10.1039/D5CC03400K
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